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The symmetry of single-molecule magnets dictates their spin quantum dynamics, influencing how such systems relax via quantum tunneling of magnetization (QTM). By reducing a system's symmetry, through the application of a magnetic field...
This dissertation presents studies on mononuclear single molecule magnets (SMMs) with magnetic properties arising from transition metal ions in trigonal bipyramidal (TBP) coordination environments. We use both experimental and...
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